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2024年9月19日 · By exploiting the mobility of the metal atoms in the liquid metal configuration and purposefully designing disordered metal catalysts, we provide insights into designing future transition...

2023年8月2日 · We show the formation of two-dimensional Ga (III) oxide islands embedded into the Cu surface in the reaction atmosphere. The islands are a few atomic layers in thickness and considerably differ...

Here, we investigated the initial stages of the Ga–Cu alloy formation on Cu (111) and Cu (001) surfaces using scanning tunneling microscopy (STM), X-ray photoelectron spectroscopy (XPS), and low energy electron diffraction (LEED).

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2023年4月20日 · A highly delocalized electron distribution intensity induced by S vacancy indicates that Cu and Ga adjacent to S vacancy form Cu–Ga metallic bond, which accelerates the photocatalytic reduction of CO 2 to C 2 H 4. The stability of the crucial intermediates (*CHOHCO) is attributed to the upshift of the d -band center of ultra-thin CGS/GS.

As a result, a highly ordered Ga–Cu N catalyst delivers an impressive ammonia faradaic efficiency (FE) of 96.48% and a stable yield of 24.36 mg h −1 −2. The fast active hydrogen (*H) generation and low eNitRR energy barrier on Ga–Cu intermetallic facets are unveiled by both theoretical calculation and dynamic experiments.